The trial polarization fields (6), (29) used in this paper depend on 2N − 2 free parameters [i.e., 2N parameter aα, bα restricted by 2 constraints (10), (11)], hence are more
general than the Hashin-Shtrikman ones used [3–5], which contain just 2 free parameters.
Therefore the new bounds are more restricting in the cases N ≥ 3. We remind the particular example of three-phase double-coated-sphere composite [1], where the parameters Aβγ α
have been determined analytically, our new bounds converge to the exact effective bulk
modulus, while the old bounds in [3, 5] do not. Note also that the trial fields (6), (29) for
the shear modulus containing 2N −2 free parameters are also more sophisticated than the
respective trial fields for the bulk modulus in [1] containing just N − 1 free parameters.
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Volume 35 Number 4
4
Vietnam Journal of Mechanics, VAST, Vol. 35, No. 4 (2013), pp. 275 – 283
CONSTRUCTION OF BOUNDS ON
THE EFFECTIVE SHEAR MODULUS OF ISOTROPIC
MULTICOMPONENT MATERIALS
Vu Lam Dong∗, Pham Duc Chinh
Institute of Mechanics, VAST, 18 Hoang Quoc Viet, Hanoi, Vietnam
∗E-mail: vldong@imech.ac.vn
Abstract. In our previous paper, we constructed bounds on the effective bulk modulus
of isotropic multicomponent composites using minimum energy principles and modi-
fied Hashin-Shtrikman polarization trial fields. In this paper, following the variational
approach, we construct more sophisticated bounds on the effective shear modulus. Ap-
plications to particular models are presented.
Keywords: Isotropic multicomponent material, effective shear elastic modulus, three-
point correlation parameters.
1. INTRODUCTION
Macroscopic (effective) elastic moduli keff and µeff of isotropic multicomponent
materials are important mechanical properties of the materials. It is difficult to find ex-
actly these moduli because of complicated micro-geometries of composites. The most well-
known estimates are the volume-weighted arithmetic or harmonic average formulae of Voigt
and Reuss (Hill first order) bounds and Hashin-Shtrikman (second order) bounds [1–5].
Pham [3] extended Hashin-Shtrikmans inequalities to incorporate a number of coefficients
depending on the fluctuation fields to improve the bounds.
In [1] we had constructed new bounds for effective bulk elastic modulus of isotropic
multicomponent materials which involve three-point correlation parameters. Continuing
the research in this direction we will use more general multi-free parameter trial fields to
construct new tight bounds on effective shear elastic properties of isotropic multicompo-
nent materials. Applications of the bounds are performed for some representative material
models.
2. CONSTRUCTION OF NEW BOUNDS
The α-component of the multicomponent composite has elastic moduli kα, µα, α =
1, ..., N . The local elastic tensor C(x) is expressible as
C(x) =
N∑
α=1
T(kα, µα)Iα(x) , x ∈ V, (1)
276 Vu Lam Dong, Pham Duc Chinh
where Iα is the indicator function
Iα(x) =
{
1, x ∈ Vα
0, x /∈ Vα
(2)
T is the isotropic fourth rank tensor with components
Tijkl(k, µ) = kδijδkl + µ(δikδjl + δilδjk −
2
3
δijδkl), (3)
δij is Kro¨necker symbol. The effective elastic moduli C
eff = T(keff , µeff ) of the composite
can be defined via the minimum energy expression [1]
ε
0 : Ceff : ε0 = inf
〈ε〉=ε0
∫
V
ε : C : εdx, (4)
while the strain field is expressible via the displacement field u(x)
ε(x) =
1
2
[∇u+ (∇u)T ]. (5)
To find the best possible upper bound on µeff from the minimum energy principle
(4), we choose the following admissible compatible strain trial field
εij = ε˜
0
ij +
N∑
α=1
[aα
1
2
(ϕα,ikε˜
0
kj + ϕ
α
,jk ε˜
0
ki) + bαψ
α
,ijklε˜
0
kl], i, j = 1, ..., 3; (6)
where ε0ij = ε˜
0
ij (ε˜
0
ii = 0) is a constant deviatoric strain; ϕ
α and ψα are the harmonic and
biharmonic potentials, Latin indices after comma designate differentiation with respective
Cartesian coordinates;
ϕα(x) =
∫
Vα
Γϕ(x− y)dy ; ∇
2ϕα(x) = δαβ , x ∈ Vβ;
Γϕ(r) = −
1
4pir
, ∇2Γϕ = δ(r);
(7)
r =| x− y | ; δ(r) is the Delta Dirac function;
ψα(x) =
∫
Vα
Γψ(x− y)dy ; ∇
4ψα(x) = δαβ , x ∈ Vβ ;
Γψ(r) = −
1
8pi
r , ∇4Γψ = δ(r).
(8)
In [3] we have introduced the three-point correlation parameters
Aβγα =
∫
Vα
ϕβαij ϕ
γα
ij dx , ϕ
βα
ij = ϕ
β
,ij −
1
vα
∫
Vα
ϕβ,ijdx,
Bβγα =
∫
Vα
ψβαijklψ
γα
ijkldx , ψ
βα
ijkl = ψ
β
,ijkl −
1
vα
∫
Vα
ψβ,ijkldx.
(9)
Construction of bounds on the effective shear modulus of isotropic multicomponent materials 277
2N free scalars aα, bα in (6) are subjected to restrictions
N∑
α=1
vαaα = 0, (10)
N∑
α=1
vαbα = 0, (11)
for the trial field (6) to satisfy the restriction 〈ε〉 = ε0 of Eq. (4). Substituting the trial field
(6) into the energy functional of Eq. (4) and taking into account (9) and the respective
expressions in [3–5], one gets
Wε =
∫
V
ε : C : εdx =
N∑
α=1
∫
vα
[
kαεiiεjj + µα
(
2εijεij −
2
3
εiiεkk
)]
dx
=
{
µV +
N∑
α=1
vαµα
[
2
3
aα +
4
15
bα +
1
9
(
aα +
2bα
5
)2]
+
N∑
α,β,γ=1
[
Aβγα
(
1
10
(kα −
2
3
µα)(aβ + bβ)(aγ + bγ) +
11
60
µαaβaγ
+
4
15
µαaβbγ −
1
15
µαbβbγ
)
+
1
5
µαbβbγB
βγ
α
]}
2ε˜0ij ε˜
0
ij,
(12)
where µV =
N∑
α=1
vαµα is Voigt arithmetic average.
We minimize the expression (12) over variable aα, bα restricted by Eqs. (10), (11)
with the help of Lagrange multipliers λ and κ and get the equations
1
3
vαµα +
vα
9
(
aα +
2bα
5
)
µα +
N∑
β,γ=1
Aαβγ
[
kγ −
2
3µγ
10
(aβ + bβ)
+
11
60
µγaβ +
2
15
µγbβ
]
− λvα = 0, α = 1, ..., N ;
(13)
2vαµα
15
+
2vαµα
45
(
aα +
2bα
5
)
+
N∑
β,γ=1
{
Aαβγ
[kγ − 23µγ
10
(aβ + bβ)
+
2µγaβ
15
−
µγbβ
15
]
+Bαβγ
µγbβ
5
}
− κvα = 0, α = 1, ..., N.
(14)
Summing Eqs. (13) multiplied by µ−1α on α from 1 to N and taking into account
Eq. (10), one gets
1
3
+
N∑
α=1
2bαvα
45
+
N∑
α,β,γ=1
Aαβγ µ
−1
α
[
aβ
(
kγ
10
+
7µγ
60
)
+ bβ
(
kγ
10
+
µγ
15
)]
− λµ−1R = 0, (15)
278 Vu Lam Dong, Pham Duc Chinh
where µR is Reuss harmonic average
µR =
(
N∑
α=1
vαµ
−1
α
)−1
. (16)
Also summing Eqs. (14) multiplied by µ−1α on α from 1 to N and taking into account Eq.
(11), one obtains
2
15
+
N∑
α=1
2aαvα
45
+
N∑
α,β,γ=1
{
Aαβγ µ
−1
α
[
aβ
(
kγ
10
+
µγ2
15
)
+bβ
(
kγ
10
−
2µγ
15
)]
+ Bαβγ µ
−1
α
µγbβ
5
}
− κµ−1R = 0.
(17)
Now substituting λ and κ from Eqs. (15) and (17) into Eqs. (13) and (14), finally
leads to equations containing only the unknown aα and bα
vµ +Aµ · a = 0. (18)
In (18) we have introduced vectors vµ, a and matrix Aµ in 2N -space
a = {a1, . . . , aN , b1, . . . , bN}
T , (19)
vµ =
{
v1
3
(µ1 − µR), . . . ,
vN
3
(µN − µR),
2v1(µ1 − µR)
15
, . . . ,
2vN(µN − µR)
15
}T
, (20)
Aµ =
{
Aµαβ
}
, α, β = 1, . . . , 2N ; (21)
where (in the following α, β = 1, ..., N ; α̂= N + α; β̂ = N + β)
Aµαβ =
vα
9
µαδαβ +
N∑
γ=1
(
Aαβγ − vαµR
N∑
δ=1
µ−1δ A
δβ
γ
)[
kγ
10
+
7µγ
60
]
,
Aµ
bαbβ
=
4vα
225
µαδαβ +
N∑
γ=1
[(
Aαβγ − vαµR
N∑
δ=1
µ−1δ A
δβ
γ
)(
kγ
10
−
2µγ
15
)
+
(
Bαβγ − vαµR
N∑
δ=1
µ−1δ B
δβ
γ
)
µγ
5
]
,
A
αbβ
=Abαβ =
2vα
45
(µαδαβ − µRvβ) +
N∑
γ=1
(
Aαβγ − vαµR
N∑
δ=1
µ−1δ A
δβ
γ
)[
kγ
10
+
µγ
15
]
.
(22)
From Eq. (18), we find the necessary solutions for aα, bα
a = −A−1µ · vµ . (23)
Construction of bounds on the effective shear modulus of isotropic multicomponent materials 279
From Eq. (12), with Eqs. (13), (14) and (23), one finds
Wε =
∫
V
ε : C : εdx =
[
µV +
1
3
N∑
α=1
vαµα
(
aα +
2bα
5
)]
2ε˜0ij ε˜
0
ij
=
(
µV + v
′
µ · a
)
2ε˜0ij ε˜
0
ij =
(
µV − v
′
µ ·A
−1
µ · vµ
)
2ε˜0ij ε˜
0
ij ,
(24)
where
v′µ =
{
v1µ1
3
, . . . ,
vNµN
3
,
2v1µ1
15
, . . . ,
2vNµN
15
}T
. (25)
From Eqs. (2), (24), finally we obtain the upper bound on the effective shear modulus
µeff ≤MUAB({kα, µα, vα}, {A
βγ
α , B
βγ
α }) = µV − v
′
µ ·A
−1
µ · vµ . (26)
To construct the lower bound on the effective shear modulus we use the minimum
complementary energy principle
σ
0 : (Ceff)−1 : σ0 = inf
〈σ〉=σ0
∫
V
σ : C−1 : σdx , (27)
where σ0 is a constant stress field, and the stress field σ should satisfy equilibrium equation
∇ · σ(x) = 0 , x ∈ V (28)
To find a lower bound on the effective shear modulus µeff from the minimum com-
plementary energy principle (27), we take the admissible equilibrated stress trial field
σij = σ˜
0
ij +
N∑
α=1
[aα(ϕ
α
,ikσ˜
0
kj + ϕ
α
,jkσ˜
0
ki − Iασ˜
0
ij)
− (aα + bα)δijϕ
α
,klσ˜
0
kl + bαψ
α
,ijklσ˜
0
kl], i, j = 1, ..., 3;
(29)
where σ0ij = σ˜
0
ij(σ˜
0
ii = 0) is a constant deviatoric stress, the free scalars aα, bα are subjected
to the same restrictions (10) and (11). Substituting the trial field (29) into (27) and
following procedure similar to that form (12) to (26), one obtains the best possible lower
bound on µeff
µeff ≥MLAB
(
{kα, µα, vα}, {A
βγ
α , B
βγ
α }
)
= (µ−1R − v¯
′
µ · A¯
−1
µ · v¯µ)
−1 , (30)
where
v¯µ =
{
−
v1
3
(µ−1
1
− µ−1V ), . . . ,−
vN
3
(µ−1N − µ
−1
V ),
2v1(µ
−1
1
− µ−1V )
15
, . . . ,
2vN (µ
−1
N − µ
−1
V )
15
}T
, (31)
v¯
′
µ =
{
−
v1µ
−1
1
3
, . . . ,−
vNµ
−1
N
3
,
2v1µ
−1
1
15
, . . . ,
2vNµ
−1
N
15
}
, (32)
A¯µ =
{
A¯µαβ
}
, α, β = 1, . . . , 2N ; (33)
280 Vu Lam Dong, Pham Duc Chinh
[in (34) α, β = 1, . . . , N ; α̂= N + α; β̂ = N + β]
A¯µαβ =
vα
9
µ−1α δαβ +
N∑
γ=1
(
Aαβγ −
vα
µV
N∑
δ=1
µδA
δβ
γ
)[
2k−1γ
45
+
7
15
µ−1γ
]
,
A¯µ
bαbβ
=
4vα
225
µ−1α δαβ +
N∑
γ=1
[(
Aαβγ −
vα
µV
N∑
δ=1
µδA
δβ
γ
)(
8k−1γ
45
−
2µ−1γ
15
)
+
(
Bαβγ −
vα
µV
N∑
δ=1
µδB
δβ
γ
)
µ−1γ
5
]
,
A¯µ
αbβ
= A¯µ
bαβ
= −
2vα
45
(
µ−1α δαβ − µ
−1
V vβ
)
+
N∑
γ=1
(
Aαβγ −
vα
µV
N∑
δ=1
µδA
δβ
γ
)[
4k−1γ
45
+
2µ−1γ
15
]
.
(34)
3. APPLICATIONS
In the case of symmetric cell material without distinct inclusion and matrix phases
[4] (Fig. 1a), the three-point correlation parameters A
βγ
α , B
βγ
α have particular forms [4, 5]
(α 6= β 6= γ 6= α)
Aβγα = vαvβvγ(f1 − f3) , A
αα
α = vα(1− vα)[(1− vα)f1 + vαf3] ,
Aαβα = vαvβ [(vα − 1)f1 − vαf3] , A
ββ
α = vαvβ [(1− vβ)f3 + vβf1] ,
Bβγα = vαvβvγ(g1 − g3) , B
αα
α = vα(1− vα)[(1− vα)g1 + vαg3] ,
Bαβα = vαvβ [(vα − 1)g1− vαg3] , B
ββ
α = vαvβ [(1− vβ)g3 + vβg1] ,
(35)
which depend on just 4 shape parameters f1, f3, g1, g3. One also has
6
7
f1 +
8
35
≥ g1 ≥
6
7
f1
f1 + f3 =
2
3
, 0 ≤ f1, f3 ≤
2
3
,
g1 + g3 =
4
5
, 0 ≤ g1, g3 ≤
4
5
.
(36)
The three-point correlation bounds (26), (30) are specialized to
MUfg ≥ µ
eff ≥MLfg, (37)
where
MUfg({kα, µα, vα}, f1, g1) =M
U
AB({kα, µα, vα}, {A
βγ
α , B
βγ
α } ∈ (35)),
MLfg({kα, µα, vα}, f1, g1) =M
L
AB({kα, µα, vα}, {A
βγ
α , B
βγ
α } ∈ (35));
(38)
and then the shape-unspecified bounds for all symmetric cell materials read
MUsym ≥ µ
eff ≥MLsym , (39)
Construction of bounds on the effective shear modulus of isotropic multicomponent materials 281
(a)
0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9
0
1
2
3
4
5
6
7
8
9
10
v
1
µ
HS
SYM
SPHE
(b)
Fig. 1. The bounds on the effective shear modulus of three-component symmetric
cell materials (SYM), compared to bounds for the specific symmetric spherical
cell materials (SPHE) and Hashin-Shtrikman (HS) bounds. (a) A symmetric cell
mixture; (b) The bounds
where
MUsym({kα, µα, vα}) = max
f1,g1∈(36)
MUfg({kα, µα, vα}, f1, g1),
MLsym({kα, µα, vα}) = min
f1,g1∈(36)
MLfg({kα, µα, vα}, f1, g1).
(40)
Numerical result for the shape-unspecified bounds on the effective shear modulus
of three-phase symmetric cell materials with same data of [1] at the range v1 = 0.1 →
0.9, v2 = v3 =
1
2(1 − v1) with k1 = 1, µ1 = 0.3, k2 = 12, µ2 = 8, k3 = 30, µ3 = 15 , are
presented in Fig. 1b, which fall inside Hashin-Shtrikman bounds for the larger class of
isotropic composites. The bounds µUs , µ
L
s (with f1 = g1 = 0) for the specific spherical cell
materials are also presented, which lie inside both presented bounds.
The next examples involve two-phase random suspensions of equisized hard spheres
(Fig. 2a ) and overlaping spheres (Fig. 3a). The parametersAβγα , B
βγ
α are expressed through
just two parameters ζ1 (or ζ2) and η1 (or η2) introduced earlier by Milton and Torquato
[6–9]
A11α = A
22
α = −A
12
α =
2
3
v1v2ζα , α = 1, 2;
B11α = B
22
α = −B
12
α =
3
10
v1v2ηα +
1
2
v1v2ζα .
(41)
The bounds (26) and (30) for the models at ranges of v2, with k1 = 1, µ1 = 0.3, k2 =
20, µ2 = 10, together with Hashin-Shtrikman bounds are projected in Figs. 2b, 3b.
282 Vu Lam Dong, Pham Duc Chinh
(a)
0.1 0.2 0.3 0.4 0.5 0.6
0
1
2
3
4
5
v
2
µ
HS
HARD
(b)
Fig. 2. Hashin-Strikman bounds (HS) and the bounds (HARD) on the elastic
shear modulus of the random suspension of equisized hard spheres. (a) A random
suspension of equisized hard spheres; (b) The bounds
(a)
0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9
0
2
4
6
8
10
v
2
µ
HS
OVERLA
(b)
Fig. 3. Hashin-Strikman bounds (HS) and the bounds (OVERLA) on the elastic
shear modulus of the random suspension of equisized overlapping spheres. (a) A
random suspension of equisized overlapping spheres; (b) The bounds
4. CONCLUSION
In this paper the authors have constructed three-point correlation bounds on the
effective shear elastic modulus of statistically isotropic N -component materials from min-
imum energy principles, using multi-free-parameter trial fields. The bounds are specified
Construction of bounds on the effective shear modulus of isotropic multicomponent materials 283
to the practical class of symmetric cell materials and random suspensions of equisized
spheres, with numerical illustrations.
The trial polarization fields (6), (29) used in this paper depend on 2N − 2 free pa-
rameters [i.e., 2N parameter aα, bα restricted by 2 constraints (10), (11)], hence are more
general than the Hashin-Shtrikman ones used [3–5], which contain just 2 free parameters.
Therefore the new bounds are more restricting in the cases N ≥ 3. We remind the particu-
lar example of three-phase double-coated-sphere composite [1], where the parameters Aβγα
have been determined analytically, our new bounds converge to the exact effective bulk
modulus, while the old bounds in [3, 5] do not. Note also that the trial fields (6), (29) for
the shear modulus containing 2N −2 free parameters are also more sophisticated than the
respective trial fields for the bulk modulus in [1] containing just N − 1 free parameters.
ACKNOWLEDGEMENT
The authors thank the financial support of Vietnam’s Nafosted, project No 107.02-
2013.20.
REFERENCES
[1] Pham Duc Chinh, Vu Lam Dong, Three-point correlation bounds on the effective bulk modulus
of isotropic multicomponent materials,Vietnam Journal of Mechanics, 34, (2012), pp. 67–77.
[2] Hashin Z., Shtrikman S., A variational approach to the theory of the elastic behaviour of
multiphase materials, J.Mech.Phys. Solids, 11, (1963), pp. 127–140.
[3] Pham D.C., Bounds on the effective shear modulus of multiphase materials, Int.J, Engng. Sci,
31, (1993), pp. 11–17.
[4] Pham D.C., Bounds for the effective conductivity and elastic moduli of fully-disordered multi-
component materials, Arch. Rational Mech. Anal, 127, (1994), pp. 191–198.
[5] Pham D.C.,Bounds for the effective properties of isotropic composite and poly-crystals, D. Sci.
Thesis , Hanoi, (1996).
[6] Milton G.W., The theory of Composites, Cambridge University Press, (2001).
[7] Torquato S.,Random heterogeneous media, New York, Springer, (2002).
[8] Pham D.C., Torquato S., Strong-contrast expansions and approximations for the effective con-
ductivity of isotropic multiphase composites, J. Appl, Phys, 94, (2003), pp. 6591–6602.
[9] Pham D.C., Three-point interpolation approximation for the macroscopic properties of isotropic
two-component materials, Philos, Mag, 87, (2007), pp. 3531–3544.
Received July 19, 2013
VIETNAM ACADEMY OF SCIENCE AND TECHNOLOGY
VIETNAM JOURNAL OF MECHANICS VOLUME 35, N. 4, 2013
CONTENTS
Pages
1. Nguyen Manh Cuong, Tran Ich Thinh, Ta Thi Hien, Dinh Gia Ninh, Free
vibration of thick composite plates on non-homogeneous elastic foundations
by dynamic stiffness method. 257
2. Vu Lam Dong, Pham Duc Chinh, Construction of bounds on the effective
shear modulus of isotropic multicomponent materials. 275
3. Dao Van Dung, Nguyen Thi Nga, Nonlinear buckling and post-buckling of
eccentrically stiffened functionally graded cylindrical shells surrounded by an
elastic medium based on the first order shear deformation theory. 285
4. N. T. Khiem, L. K. Toan, N. T. L. Khue, Change in mode shape nodes of
multiple cracked bar: II. The numerical analysis. 299
5. Tran Van Lien, Trinh Anh Hao, Determination of mode shapes of a multiple
cracked beam element and its application for free vibration analysis of a multi-
span continuous beam. 313
6. Phan Anh Tuan, Pham Thi Thanh Huong, Vu Duy Quang, A method of skin
frictional resistant reduction by creating small bubbles at bottom of ships. 325
7. Nguyen Thoi Trung, Bui Xuan Thang, Ho Huu Vinh, Lam Phat Thuan,
Ngo Thanh Phong, An effective algorithm for reliability-based optimization
of stiffened Mindlin plate. 335
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