Hơn ba thập kỉ trƣớc, Fazekas và Anderson đã tìm ra một trong các trạng thái cơ bản của
spin, trạng thái spin lỏng lƣợng, với nhiều đặc điểm kì lạ. Sau nhiều năm tìm kiếm, gần đây đã
xuất hiện các thí nghiệm nhƣ những minh chứng rõ ràng về sự tồn tại của trạng thái này ở các hệ
frustrated spin. Đáng tiếc là các mô hình vi mô mô tả sự tồn tại của trạng thái này vẫn còn khá
hiếm. May mắn là, với sự phát triển mạnh mẽ trong hơn thập kỉ qua của hệ thống lí thuyết đã mở
ra bƣớc tiến mới trong nghiên cứu sử dụng phƣơng pháp mô phỏng bằng sử dụng máy tính áp
dụng cho các hệ lớn và phức tạp. Trong công trình này, chúng tôi sử dụng phƣơng pháp mô
phỏng Monte Carlo lƣợng tử để khảo sát tính chất vật lí của trạng thái cơ bản trong mô hình nút
mạng Kagome hai chiều spin -1/2 XY với tƣơng tác trao đổi vòng bốn nút. Chúng tôi đã phát
hiện quá trình chuyển pha loại hai từ trạng thái siêu lỏng sang trạng thái spin lỏng lƣợng tử đối
xứng Z2. Bên cạnh đó, trạng thái spin lỏng lƣợng tử cũng đƣợc chúng tôi mô tả rõ ràng thông
qua các tham số trật tự đặc trƣng nhƣ hệ số cấu trúc tĩnh spin-spin, các hệ số cấu trúc khung bốn
đỉnh. Đáng chú ý, chúng tôi đã tìm thấy số mũ dị thƣờng trong chuyển pha ηXY* ≈ 1.325 lớn
khác thƣờng so với hệ số tìm thấy trong mô hình tổng quát 3D XY. Chúng tôi không tìm thấy tín
hiệu của sự xuất hiện pha siêu rắn xen giữa các trạng thái siêu lỏng và trạng thái QSL
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Journal of Science and Technology 54 (1A) (2016) 17-24
THE PHYSICS OF SPIN-1/2 XY MODEL WITH FOUR-SITE
EXCHANGE INTERACTION ON THE KAGOME LATTICE
Nguyen Thi Kim Oanh
1
, Pham Thanh Dai
1
, Dang Dinh Long
1, 2, *
1
VNU-University of Engineering and Technology, 144 Xuan Thuy, Cau Giay, Hanoi
2
University of Ulsan, 93, Daehak-ro, Nam-gu, Ulsan, Korea
*
Email: longdd@gmail.com
Received: 19 August 2015; Accepted for publication: 25 October 2015
ABSTRACT
The quantum spin liquid (QSL) state, proposed more than three decades ago by Fazekas and
Anderson remains surprisingly elusive. Although recent experiments provide a strong evidence of
their existence in the frustrated spin systems, the microscopic model for this state is still rare. The
extensive theoretical framework, developed over decades, continues to extend further motivated
by these and other discoveries from large-scale computer simulations of a relatively small number
of models. In this work, we discuss the physics of the ground-state phase diagram of a two-
dimensional Kagome lattice spin-1/2 XY model with a four-site ring-exchange interaction using
quantum Monte Carlo simulation. We found the second order phase transition from superfluid
state to a Z2 quantum spin liquid phase driven by the four-site ring exchange interaction. We have
characterized the QSL by its vanishing order parameters such as the spin-spin structure factor, the
plaquette-plaquette structure factor. Moreover, we have found the large anomalous exponent ηXY*
≈ 1.325 which belongs to a different universality class other than 3D XY universality class. There
is no signal of supersolid phase intervening between the superfluid state and QSL state.
Keywords: Quantum Spin Liquid, Kagome Lattice, Quantum Monte Carlo, Ring Exchange
Model, critical exponents.
1. INTRODUCTION
Although Fazekas and Anderson [1] proposed an idea of quantum spin liquid (QSL) state
three decades ago, recent neutron scattering experiments on the spin-1/2 Kagome lattice
ZnCu3(OH)6Cl2 (Herbertsmithite) [2] and prochlore compounds mapping to Kagome ices,
particularly Tb2Ti2O7, Yb2Ti2O7, Pr2Zr2O7, and Pr2Sn2O7 , provide the significant evidences of its
existence [3, 4, 5]. The extensive study of QSL is expected to have a large impact on the future
computing technology like a topological quantum computing [6, 7]. It is believed that the
geometric frustration is a main ingredient for a microscopic model of QSL state. The theoretical
framework has developed for three decades, and still needs to explore further due to the
complexity of QSL phase structure [8, 9]. The significant motivation came from the power of
large-scale computer simulation after Yan et al. has recently applied density matrix
Nguyen Thi Kim Oanh, Pham Thanh Dai, Dang Dinh Long
18
renormalization group to explain the existence of QSL in the ground state of the Kagome-lattice
Heisenberg antiferromagnet [10]. However, the study of a gapped QSL using Quantum Monte
Carlo simulation of the honeycomb lattice Hubbard model at half filling predicted some
contradiction [11]. The difficulty in finding models for Quantum Monte Carlo is the fact that the
frustration typically leads to the infamous sign problem. Fortunately, Balents et al. proposed a
sign-problem free Hamiltonian of spins on Kagome lattice exhibited the QSL state which can be
attacked by Quantum Monte Carlo simulation [12]. Recently Dang et al. has also utilized the
large-scalable Quantum Monte Carlo to extract the signals of QSL in Kagome lattice [13]. The
interesting transition to QSL state characterized by an exotic XY* universality class, namely XY*
universality class, caused by the condensation of bosonic spinons, which has unfortunately not
been addressed yet. Although the neutron scattering experiments in Cs2CuCl4 suggested the large
anomalous dimension ηXY* in the range of 0.7 - 1.0 [14, 15].
More interestingly, Bloch et al. [16] has proposed a unique experiment setting for quantum
simulation of the artificial structure in optical lattice with the high degree of controllability. And,
Buchler et al. [17] have also provided an experimental design of a ring exchange interaction for
ultracold atoms in 2D optical lattice. These settings make the ring exchange model more reliable
and controllable.
In this paper, we carry out a study of Z2 QSL phase using a model with competition between
two purely kinetic terms, namely spin-1/2 model with four-site ring exchange interaction in the
Kagome lattice. A large scale finite temperature Quantum Monte Carlo (QMC) simulation is
applied to characterize the different quantum phases as well as their transition. We find that there
is a second order quantum phase transition between the superfluid and quantum spin liquid state
driven by the ring exchange interaction. A significant large anomalous critical exponent ηXY* ≈
1.325 is qualitatively consistent with the classical Monte Carlo simulation [18] as well as the
broad line shapes seen in experiment of Cs2CuCl4 [14,15].
Moreover, the geometrical frustration does not typically induce the supersolid state [19]. In
this study, we have also supported to this claim, i.e. there is no signature of supersolid state
intervening between the superfluid state and QSL state.
2. QUANTUM MONTE CARLO SIMULATION
The well-known model of spin-1/2 XY model with four-site exchange interaction
Hamiltonian reads:
ij ijkl
ij ijkl
H J B K P (1)
where denotes a pair of nearest neighbor sites and denotes the sites on the corners of
a bow-tie plaquette on 2D Kagome lattice, J factor is the nearest neighbor coupling strength and
K factor is the foursite ring exchange strength; the bond operator ( )
ij i j i j
B S S S S describes the
nearest neighbor XY exchange interaction; and the plaquette operator ( )
ij i j k l i j k l
B S S S S S S S S
(the labelling rule is defined in Figure 1 a) describes the four-site ring exchange interaction
(Figure 1b). Hamiltonian (1), in short J-K model, can be mapped into the Bose-Hubbard model
using the Holstein-Primakoff transformation. In the bosonic language, the bond operator
represents the hopping energy between two nearest neighbor interaction whereas the plaquette
operator represents the ring hopping around the 4 sites on Kagome lattice (Figure 1 c).
Interestingly, two terms J and K are all purely kinetic energy which is different from the regular
The physics of spin -1/2 XY model with four-site exchange
19
model in which the exotic phase driven by the competition between the kinetic and potential
energy. For simplicity, J = 1 has been chosen for energy scale. The same version of Hamiltonian
(1) , except for the square lattice XY ring exchange model, has shown the deconfined quantum
critical point between a superfluid and valence-bond-solid (VBS). VBS has shown a non-
magnetic order but its plaquette correlation displays a long range feature, meaningfully, there is
no QSL state in the square lattice model.
Figure 1 (a) Kagome lattice and a labeling convention for the indices of the bond operator Bij and plaquette
operator Pijkl. Two primitive vectors 1 2,a a are shown. (b) Two spin plaquette configuration describes the
four-site spin ring exchange. (c) Particle-hole configuration represents the plaquette configuration in the
bosonic language.
We investigate the J-K model (1) using QMC technique namely the stochastic series
expansion (SSE) algorithm [20, 21] which does not suffer from sign problem. The system size
are defined as
1 1 1
L n a and 2 2 2L n a with two primitive vectors 1 2 1a a (shown in Figure
1.a). Moreover, the total number of sites in the simulation cell is defined as
1 2
3
s
N n n . In
principle, we can make
1 2
n n to investigate the structure as a ladder, we however take
1 2
n n L for simplicity.
The QMC simulations have been carried out at finite temperature but the ground state
phase diagram can be extrapolated at very low temperature. In other words, the imaginary time β
≈ L has been fixed during the simulations. The finite temperature phase diagram could be
addressed in the other MC studies. We characterize the various phases in this model by
investigating the spin stiffness as well as the spin and plaquette structure factors. The spin
stiffness is defined as:
2
2
1 ( )
S
s
E
N
(2)
where is a twist in the periodic boundary of the lattice, hence the spin stiffness is the energy
( )E response to the twist. In bosonic language, it is a superfluid density induced by the
winding numbers in imaginary time space configuration. The spin structure factor can be
calculated from the Fourier transformation of the z-component,
, ,
(1 / 2)
z z
k l k l
S with
,
1
z
k l
, of
the spin-spin correlation function
1
1
1 1
( ) ( )
4
nz z z z
k l k lp
S S p p
n
with n is the number of non-
identity operators in the Monte Carlo - SSE operator list at the wavevector q=(qx, qy):
Nguyen Thi Kim Oanh, Pham Thanh Dai, Dang Dinh Long
20
( ).
,
1
( , ) k l
i r r q z z z z
s x y k l k l
k l
S q q e S S S S
N
(3)
where, k and l are lattice sites and ri=(xi, yi) is the lattice coordinate. Similarly, the plaquette
structure factor reads:
( ).
,
1
( , ) m n
i r r q z z z z
p x y m n m n
m n
q q e P P P P
N
B (4)
where Pm, Pn are the plaquette operator.
3. RESULTS AND DISCUSSION
Since QSL does not have a regular order parameter as the description in Landau theory of
phase transition, the characteristic of the various phases in J-K model (1) must be investigated
carefully. We first look at the finite size scaling behavior. In our simulation, we study the
superfluid stiffness (2) using the general scaling form near the quantum critical transition point [22]:
1/
( , / )
S
z z
S
L F tL L (5)
where,
S
F is a universal scaling function, and
c
t K K , L is the linear system size, is the
inverse temperature or the imaginary time, z = 1 is the dynamical critical exponent, and = 0.43
is the correlation length exponent [19] which is slightly different from the typical 3D XY
universality class. Our simulation shows the superfluid density vanishing with increasing the
ring exchange interaction which suggests a second order phase transition. Now, we apply the
scaling relation (5) and plot
z
S L as a function of ct K K to determine the critical point cK =
21.8.
Figure 2 Collapse of the scaling function for superfluid density
z
S
L at ground state as a function of four-
site ring exchange. The critical value of the ring exchange Kc = 21.8 separates the quantum spin liquid
with superfluid state. Inset: ground state diagram of Hamiltonian (1) with superfluid phase (SF) and
quantum spin liquid (QSL) separated by the critical ring exchange interaction.
Figure 2 shows that all the curves collapse into a single curve for the conventional 3D XY
universality class. As the result, we have found the large anomalous exponent ηXY* ≈ 1.325 using
the scaling relation [22]:
The physics of spin -1/2 XY model with four-site exchange
21
*
*2 ( 2 )
XY
d z
where,
*
= 0.5 is the critical exponent, d = 2 is the dimensionality for 2D system (taken from
the well-known 3D XY universality class). It is worthy to note that an anomalous exponent
belonging to the 3D XY universality class ηXY ≈ 0.04 which is much smaller than our finding.
This can be explained through the condensation of bosonic spinons at the transition. The
transition from superfluid to insulating phase with the large anomalous critical exponent
suggests that the insulating phase is Z2 quantum spin liquid.
In order to rule out the other possibilities of the order phase such as the solid state or the
valence bond state, we make a further investigation by examining the spin structure factor.
Figure 3 shows the spin structure factor as a function of 1/Ls ( 3sL L L ) of an insulating state
with K = 26 at the wavevector qmax = (0, 4 / 3 ) corresponding to the Bragg peak required for
the long range order such as solid order in crystal. The spin structure factor dies off with an
increase of the system size and approaches zero in the thermodynamic limit. This feature signals
a short range correlation and rule out the possibility of having solid order with a regular broken
symmetry. It immediately rules out the possibility of supersolid phase in this system as well.
Figure 3 Spin structure S(qmax) at a certain wave vector qmax = (0, 4 / 3 ) as a function of 1/Ls
3
s
L L L ) for an insulating state with K = 26.
Figure 4 Plaquette structure factor B(qmax) at a certain wave vector qmax = (0, 15 / 6 3 ) as a function
of 1/Ls ( 3sL L L ) for an insulating state with K = 26.
Nguyen Thi Kim Oanh, Pham Thanh Dai, Dang Dinh Long
22
In Figure 4, we illustrate the plaquette structure factor as a function of the inverse system
size 1/Ls. Similar to the spin structure factor, the plaquette structure factor at wavevectorqmax = (0,
15 / 6 3 ) vanishes in the thermodynamic limit. This again shows no evidence of valence bond
state for the insulating phase.
4. CONCLUSIONS
In conclusion, we have studied the ground state phase diagram of the Kagome lattice spin-
1/2 XY model with a four-site ring exchange model using the modified SSE large-scale quantum
Monte Carlo simulation. We have shown the second order transition from superfluid state to
quantum spin liquid state belonging to the exotic 3D XY* universality class. The regular order
structure such as the solid or spin wave order and valence bond order has not been observed in
this system. We have also confirmed that the supersolid state does not exist in this frustrated
system. This finding is consistent with the previous study [18]. Significantly, the quantum
critical point has a dynamical exponent z = 1, the correlation length exponent = 0.44 and large
anomalous critical dimension ηXY* ≈ 1.325. It is very interesting to point out that several system
such as CsCuCl4 even shows the spin liquid state at finite temperature instead of its appearance
in the ground state phase diagram [14, 15]. This suggests a further investigation of the finite
temperature phase diagram which is also accessible with SSE simulation. Moreover, the
interaction should be taken into account since this may give rise many interesting physics
mechanism , i.e. a vison-condensation transition as well as the less computational resource to
characterize the phase diagram with SSE simulation.
Acknowledgements This work has been supported by Vietnam National University, Hanoi (VNU), under
Project No. QG.15.24 and Long Dang is grateful to the hospitality of University of Ulsan, Korea.
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TÓM TẮT
TÍNH CHẤT VẬT LÍ CỦA MÔ HÌNH SPIN -1/2 XY VỚI TƢƠNG TÁC TRAO ĐỔI TRÊN
BỐN VỊ TRÍ VÒNG TRONG MẠNG KAGOME
Nguyễn Thị Kim Oanh1, Phạm Thanh Đại1, Đặng Đình Long1, 2, *
1Đại học Công nghệ - ĐHQG Hà Nội, 144 Xuân Thủy, Cầu Giấy, Hà Nội
2Đại học Ulsan, 93, Daehak-ro, Nam-gu, Ulsan, Hàn Quốc
*
Email: longdd@gmail.com
Nguyen Thi Kim Oanh, Pham Thanh Dai, Dang Dinh Long
24
Hơn ba thập kỉ trƣớc, Fazekas và Anderson đã tìm ra một trong các trạng thái cơ bản của
spin, trạng thái spin lỏng lƣợng, với nhiều đặc điểm kì lạ. Sau nhiều năm tìm kiếm, gần đây đã
xuất hiện các thí nghiệm nhƣ những minh chứng rõ ràng về sự tồn tại của trạng thái này ở các hệ
frustrated spin. Đáng tiếc là các mô hình vi mô mô tả sự tồn tại của trạng thái này vẫn còn khá
hiếm. May mắn là, với sự phát triển mạnh mẽ trong hơn thập kỉ qua của hệ thống lí thuyết đã mở
ra bƣớc tiến mới trong nghiên cứu sử dụng phƣơng pháp mô phỏng bằng sử dụng máy tính áp
dụng cho các hệ lớn và phức tạp. Trong công trình này, chúng tôi sử dụng phƣơng pháp mô
phỏng Monte Carlo lƣợng tử để khảo sát tính chất vật lí của trạng thái cơ bản trong mô hình nút
mạng Kagome hai chiều spin -1/2 XY với tƣơng tác trao đổi vòng bốn nút. Chúng tôi đã phát
hiện quá trình chuyển pha loại hai từ trạng thái siêu lỏng sang trạng thái spin lỏng lƣợng tử đối
xứng Z2. Bên cạnh đó, trạng thái spin lỏng lƣợng tử cũng đƣợc chúng tôi mô tả rõ ràng thông
qua các tham số trật tự đặc trƣng nhƣ hệ số cấu trúc tĩnh spin-spin, các hệ số cấu trúc khung bốn
đỉnh. Đáng chú ý, chúng tôi đã tìm thấy số mũ dị thƣờng trong chuyển pha ηXY* ≈ 1.325 lớn
khác thƣờng so với hệ số tìm thấy trong mô hình tổng quát 3D XY. Chúng tôi không tìm thấy tín
hiệu của sự xuất hiện pha siêu rắn xen giữa các trạng thái siêu lỏng và trạng thái QSL.
Từ khóa: spin lỏng lƣợng tử, mạng Kagome, Monte Carlo lƣợng tử, mô hình trao đổi vòng, chỉ
số tới hạn.
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